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It was applied for the murder of the Lord President. For example, the Fourth Doctor, framed by the Master for the death of the President, was threatened by this kind of death sentence. The Doctor believed vaporisation without legal representation were against the Constitution. (TV: The Deadly Assassin)
Similar techniques Edit
By the time of Borusa's presidency, ordinarily it wasn't made provision for executions, except for severe cases threatening collective security, in which molecular dispersal was the employed method. (TV: Arc of Infinity)